Molecular Water Oxidation Catalysis: A Key Topic for New Sustainable Energy Conv

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Molecular Water Oxidation Catalysis

by Antoni Llobet

Photocatalytic water splitting is a promising strategy for capturing energy from the sun by coupling light harvesting and the oxidation of water, in order to create clean hydrogen fuel.

FORMAT Hardcover LANGUAGE English CONDITION Brand New

Publisher Description

Photocatalytic water splitting is a promising strategy for capturing energy from the sun by coupling light harvesting and the oxidation of water, in order to create clean hydrogen fuel. Thus a deep knowledge of the water oxidation catalysis field is essential to be able to come up with useful energy conversion devices based on sunlight and water splitting. Molecular Water Oxidation Catalysis: A Key Topic for New Sustainable Energy Conversion Schemes presents a comprehensive and state-of-the-art overview of water oxidation catalysis in homogeneous phase, describing in detail the most important catalysts discovered today based on first and second row transition metals. A strong emphasis is placed on the description of their performance, as well as how they work from a mechanistic perspective. In addition, a theoretical description of some of the most relevant catalysts based on DFT are presented, as well as a description of related natural systems, such as the oxygen evolving system of photosystem II and the heme chlorite-dismutase. This book is a valuable resource for researchers working on water oxidation catalysis, solar energy conversion and artificial photosynthesis, as well as for chemists and materials scientists with a broad interest in new sustainable energy conversion schemes.

Author Biography

Professor Dr. Antoni Llobet, Institute of Chemical Research of Catalonia (ICIQ) and Universitat Autònoma de Barcelona, Spain
Professor Llobet is one of the world leaders on water oxidation catalysis. He has been working in the field of redox catalysis for 25 years; his research interests include the development of tailored transition metal complexes as catalysts for selective organic and inorganic transformations including the oxidation of water to molecular dioxygen, supramolecular catalysis, the activation of C-H and C-F bonds, and the preparation low molecular weight complexes as models of the active sites of oxidative metalloproteins.
In 2000, Professor Llobet received the Distinction Award from Generalitat de Catalunya for Young Scientists and in 2011 he was awarded the Bruker Prize in Inorganic Chemistry from the Spanish Royal Society of Chemistry (RSEQ). He is the author of over 120 research publications.

Table of Contents

List of Contributors xi Preface xv 1. Structural Studies of Oxomanganese Complexes for Water Oxidation Catalysis 1
Ivan Rivalta, Gary W. Brudvig, and Victor S. Batista 1.1 Introduction 1 1.2 Structural Studies of the OEC 2 1.3 The Dark-Stable State of the OEC 4 1.4 Biomimetic Oxomanganese Complexes 6 1.5 Base-Assisted O–O Bond Formation 7 1.6 Biomimetic Mn Catalysts for Artificial Photosynthesis 8 1.7 Conclusion 11 Acknowledgments 12 References 12 2. O–O Bond Formation by a Heme Protein: The Unexpected Efficiency of Chlorite Dismutase 15
Jennifer L. DuBois 2.1 Introduction 15 2.2 Origins of O2-Evolving Chlorite Dismutases (Clds) 15 2.3 Major Structural Features of the Proteins and their Active Sites 16 2.4 Efficiency, Specificity, and Stability 20 2.5 Mechanistic Insights from Surrogate Reactions with Peracids and Peroxide 22 2.6 Possible Mechanisms 23 2.7 Conclusion 25 Acknowledgements 25 References 25 3. Ru-Based Water Oxidation Catalysts 29
Laia Francàs, Roger Bofill, Jordi García-Antón, Lluis Escriche, Xavier Sala and Antoni Llobet 3.1 Introduction 29 3.2 Proton-Coupled Electron Transfer (PCET) and Water Oxidation Thermodynamics 31 3.3 O–O Bond Formation Mechanisms 33 3.4 Polynuclear Ru Water Oxidation Catalysts 34 3.5 Mononuclear Ru WOCs 40 3.6 Anchored Molecular Ru WOCs 42 3.7 Light-Induced Ru WOCs 43 3.8 Conclusion 45 Acknowledgments 46 References 46 4. Towards the Visible Light-Driven Water Splitting Device: Ruthenium Water Oxidation Catalysts with Carboxylate-Containing Ligands 51
Lele Duan, Lianpeng Tong, and Licheng Sun 4.1 Introduction 51 4.2 Binuclear Ru Complexes 52 4.3 Mononuclear Ru Complexes 54 4.3.1 Ru–O2N–N3 Analogs 55 4.3.2 Ru–O2N2–N2 Analogs 57 4.4 Homogeneous Light-Driven Water Oxidation 68 4.4.1 The Three-Component System 68 4.4.2 The Supramolecular Assembly Approach 69 4.5 Water Oxidation Device 72 4.5.1 Electrochemical Water Oxidation Anode 72 4.5.2 Photo-Anode for Water Oxidation 74 4.6 Conclusion 75 References 75 5. Water Oxidation by Ruthenium Catalysts with Non-Innocent Ligands 77
Tohru Wada, Koji Tanaka, James T. Muckerman, and Etsuko Fujita 5.1 Introduction 77 5.2 Water Oxidation Catalyzed by Dinuclear Ruthenium Complexes with NILs 81 5.3 Water Oxidation by Intramolecular O–O Coupling with [RuII2 (

Details ISBN1118413377 Year 2014 ISBN-10 1118413377 ISBN-13 9781118413371 Format Hardcover Place of Publication New York Country of Publication United States DEWEY 541.393 Subtitle A Key Topic for New Sustainable Energy Conversion Schemes Short Title MOLECULAR WATER OXIDATION CATA Language English Media Book Publication Date 2014-05-30 Illustrations illustrations Edition 1st Author Antoni Llobet UK Release Date 2014-05-30 AU Release Date 2014-06-03 NZ Release Date 2014-06-03 Pages 304 Publisher John Wiley & Sons Inc Imprint John Wiley & Sons Inc Audience Professional & Vocational US Release Date 2014-05-30

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TheNile_Item_ID:136201043;
  • Condition: Brand New
  • ISBN-13: 9781118413371
  • Book Title: Molecular Water Oxidation Catalysis
  • ISBN: 9781118413371
  • Publication Year: 2014
  • Type: Textbook
  • Format: Hardcover
  • Language: English
  • Publication Name: Molecular Water Oxidation Catalysis: a Key Topic for New Sustainable Energy Conversion Schemes
  • Item Height: 251mm
  • Author: Antoni Llobet
  • Publisher: John Wiley & Sons Inc
  • Item Width: 168mm
  • Subject: Chemistry
  • Item Weight: 648g
  • Number of Pages: 282 Pages

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